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Performance and short-term stability of single chamber SOFCs based on La0.9Sr0.1Ga0.8Mg0.2O3-d electrolyte
dc.contributor.author | Morales Comas, Miguel |
dc.contributor.author | Roa Rovira, Joan Josep |
dc.contributor.author | Tartaj, Jesus |
dc.contributor.author | Segarra Rubi, Merce |
dc.contributor.other | Universitat Politècnica de Catalunya. Departament de Ciència dels Materials i Enginyeria Metal·lúrgica |
dc.date.accessioned | 2012-12-13T10:40:14Z |
dc.date.created | 2012-10-15 |
dc.date.issued | 2012-10-15 |
dc.identifier.citation | Morales, M. [et al.]. Performance and short-term stability of single chamber SOFCs based on La0.9Sr0.1Ga0.8Mg0.2O3-d electrolyte. "Journal of power sources", 15 Octubre 2012, vol. 216, p. 417-424. |
dc.identifier.issn | 0378-7753 |
dc.identifier.uri | http://hdl.handle.net/2117/17125 |
dc.description.abstract | In the present work, the performance of La0.9Sr0.1Ga0.8Mg0.2O3 (LSGM) electrolyte-supported SOFCs was evaluated under single-chamber conditions. For this purpose, two single cells, one with and the other without Sm0.2Ce0.8O3−δ (SDC) buffer layer between anode and electrolyte, were studied in order to determine and compare the performance and short-term stability of cells under single-chamber conditions. The reactivity of the Ni-SDC anode with SDC (for the cell with buffer layer) and the LSGM electrolyte (for the cell without buffer layer) were studied by X-ray diffraction. The reaction between Ni and LSGM during anode sintering and cell operation leads to a substantial loss in the cell performance when no buffer layer is present. As a result, maximum power densities of 246 and 132 mW cm−2 were obtained for the buffered and non-buffered cells respectively, at 800 °C, under optimized gas composition (CH4/O2 = 1.2) and a total flow rate of 400 ml min−1. After 55 h operating at 750 °C and 6 thermal cycles, the performances of both cells were decreased around 25–30 mW cm−2. |
dc.format.extent | 8 p. |
dc.language.iso | eng |
dc.rights | Attribution-NonCommercial-NoDerivs 3.0 Spain |
dc.rights.uri | http://creativecommons.org/licenses/by-nc-nd/3.0/es/ |
dc.subject | Àrees temàtiques de la UPC::Enginyeria dels materials |
dc.subject.lcsh | Fuel cells |
dc.title | Performance and short-term stability of single chamber SOFCs based on La0.9Sr0.1Ga0.8Mg0.2O3-d electrolyte |
dc.type | Article |
dc.subject.lemac | Piles de combustible |
dc.identifier.doi | 10.1016/j.jpowsour.2012.05.076 |
dc.description.peerreviewed | Peer Reviewed |
dc.relation.publisherversion | http://www.sciencedirect.com/science/article/pii/S0378775312009457 |
dc.rights.access | Restricted access - publisher's policy |
local.identifier.drac | 11067349 |
dc.description.version | Postprint (published version) |
dc.date.lift | 10000-01-01 |
local.citation.author | Morales, M.; Roa, J.; Tartaj, J.; Segarra, M. |
local.citation.publicationName | Journal of power sources |
local.citation.volume | 216 |
local.citation.startingPage | 417 |
local.citation.endingPage | 424 |
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