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Modelling the release of Mo, Tc, Ru and Rh from high burnup spent nuclear fuel at alkaline and hyperalkaline pH

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10.1557/s43580-023-00752-6
 
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hdl:2117/400104

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Giménez Izquierdo, Francisco JavierMés informacióMés informacióMés informació
Pablo Ribas, Joan deMés informacióMés informacióMés informació
García Gómez, SoniaMés informacióMés informacióMés informació
Serrano Purroy, Daniel
Iglesias Pérez, Luis
Clarens Blanco, Frederic
Martínez Torrents, Albert
Document typeArticle
Defense date2023-12-30
PublisherCambridge University Press
Rights accessOpen Access
Attribution 4.0 International
This work is protected by the corresponding intellectual and industrial property rights. Except where otherwise noted, its contents are licensed under a Creative Commons license : Attribution 4.0 International
Abstract
The present work shows experimental data on the release of some radionuclides that are forming the so-called e particles in the spent nuclear fuel (SNF): Mo, Tc, Ru and Rh. The leaching experiments were carried out with a 60 GWd·t-1 burnup SNF at two different pH values, 8.4 and 13.2, and under oxidizing conditions. The modelling of the data showed that the higher release of Mo, Tc, Ru and Rh at pH 13.2 could be due to the higher dissolution rate of the e-particles.
CitationGimenez, F. [et al.]. Modelling the release of Mo, Tc, Ru and Rh from high burnup spent nuclear fuel at alkaline and hyperalkaline pH. "MRS Advances", 30 Desembre 2023, 
URIhttp://hdl.handle.net/2117/400104
DOI10.1557/s43580-023-00752-6
ISSN2059-8521
Publisher versionhttps://link.springer.com/article/10.1557/s43580-023-00752-6
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  • Doctorat en Enginyeria de Processos Químics - Articles de revista [141]
  • R2EM - Resource Recovery and Environmental Management - Articles de revista [252]
  • Departament d'Enginyeria Química - Articles de revista [2.434]
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