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Renewable terephthalate polyesters from carbohydrate-based bicyclic monomers

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10.1039/C3GC42394H
 
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hdl:2117/22945

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Muñoz Guerra, SebastiánMés informacióMés informacióMés informació
Lavilla Aguilar, Cristina
Japu, Cristina
Martínez de Ilarduya Sáez de Asteasu, Domingo AntxonMés informacióMés informacióMés informació
Document typeArticle
Defense date2014-04-01
Rights accessRestricted access - publisher's policy
Attribution-NonCommercial-NoDerivs 3.0 Spain
This work is protected by the corresponding intellectual and industrial property rights. Except where otherwise noted, its contents are licensed under a Creative Commons license : Attribution-NonCommercial-NoDerivs 3.0 Spain
Abstract
Poly(alkylene terephthalate)s, PET and PBT in particular, are materials of great relevance and growing projection in the thermoplastic field but are today almost totally produced from fossil resources. The current huge consumption of these polyesters necessitates urgent actions addressed to make them renewable by using naturally-occurring raw materials. Among the different approaches that are being followed to develop bio-based poly(terephthalate)s, the use of bicyclic carbohydrate-derived difunctional compounds as building-blocks is receiving much attention in the last few years because partially renewable polyesters with high Tg may be thus obtained. This review presents a critical account of the terephthalate homopolymers and copolymers that have been synthesized using the two types of carbohydrate-based bicyclic monomers, isohexides and diacetals, explored to date. The properties displayed by the novel bio-based poly(terephthalate)s in relation to the bicyclic structure of the used monomers are comparatively reviewed and their potential as emergent materials for thermoplastic applications is evaluated.
CitationMuñoz, S. [et al.]. Renewable terephthalate polyesters from carbohydrate-based bicyclic monomers. "Greenchemistry", 01 Abril 2014, vol. 16, núm. 4, p. 1716-1739. 
URIhttp://hdl.handle.net/2117/22945
DOI10.1039/C3GC42394H
ISSN1463-9262
Publisher versionhttp://pubs.rsc.org/en/content/articlelanding/2014/gc/c3gc42394h#!divAbstract
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  • POL - Polímers Industrials Avançats i Biopolímers Tecnològics - Articles de revista [125]
  • Departament d'Enginyeria Química - Articles de revista [2.446]
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