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dc.contributor.authorSaemisch, Lisa
dc.contributor.authorLiebel, Matz
dc.contributor.authorHulst, Niek F. van
dc.date.accessioned2020-07-15T14:22:09Z
dc.date.issued2020-01-16
dc.identifier.citationSaemisch, L.; Liebel, M.; Hulst, N. F. V. Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection. "Nanoscale", 16 Gener 2020, vol. 12, núm. 3723.
dc.identifier.urihttp://hdl.handle.net/2117/192976
dc.description.abstractTraditionally, the nanoscale interaction between single photon emitters and plasmonic nanostructures is studied by relying on deterministic, near-perfect, nanoscale-control, either top-down or bottom-up. However, these approaches are ultra-low throughput thus rendering systematic studies difficult and timeconsuming. Here, we show a highly parallelised far-field tactic, combining multiplexed super-resolution fluorescence localization microscopy and data-driven statistical analysis, to study near-field interactions between gold nanorods and single molecules, even at bulk concentrations. We demonstrate that ensemble-level single molecule detection allows separating individual emitters according to their coupling strength with tailored resonant structures, which ultimately permits the reconstruction of super-resolved 2D interaction maps around individual nanoantennas.
dc.format.extent8 p.
dc.language.isoeng
dc.publisherRoyal Society of Chemistry
dc.rightsAttribution-NonCommercial-NoDerivs 3.0 Spain
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/3.0/es/
dc.subjectÀrees temàtiques de la UPC::Física
dc.subject.lcshOptical antennas
dc.subject.othernanoantennas
dc.titleIsolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
dc.typeArticle
dc.subject.lemacAntenes òptiques
dc.identifier.doi10.1039/c9nr08833d
dc.description.peerreviewedPeer Reviewed
dc.relation.publisherversionhttps://pubs.rsc.org/en/content/articlelanding/2020/nr/c9nr08833d#!divAbstract
dc.rights.accessRestricted access - publisher's policy
dc.description.versionPostprint (author's final draft)
dc.relation.projectid670949-LightNet
dc.date.lift2021-01-16
local.citation.publicationNameNanoscale
local.citation.volume12
local.citation.number3723


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Except where otherwise noted, content on this work is licensed under a Creative Commons license : Attribution-NonCommercial-NoDerivs 3.0 Spain