WSe2 as transparent top gate for infrared near-field microscopy
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2D-SIPC - Two-dimensional quantum materials and devices for scalable integrated photonic circuits (EC-H2020-820378)
GrapheneCore3 - Graphene Flagship Core Project 3 (EC-H2020-881603)
TOPONANOP - Topological nano-photonics (EC-H2020-726001)
ICFOstepstone - ICFOstepstone PhD Programme for Early-Stage Researchers in Photonics (EC-H2020-665884)
Abstract
Independent control of carrier density and out-of-plane displacement field is essential for accessing novel phenomena in two-dimensional (2D) material heterostructures. While this is achieved with independent top and bottom metallic gate electrodes in transport experiments, it remains a challenge for near-field optical studies as the top electrode interferes with the optical path. Here, we characterize the requirements for a material to be used as the top-gate electrode and demonstrate experimentally that few-layer WSe2 can be used as a transparent, ambipolar top-gate electrode in infrared near-field microscopy. We carry out nanoimaging of plasmons in a bilayer graphene heterostructure tuning the plasmon wavelength using a trilayer WSe2 gate, achieving a density modulation amplitude exceeding 2 × 1012 cm–2. The observed ambipolar gate–voltage response allows us to extract the energy gap of WSe2, yielding a value of 1.05 eV. Our results provide an additional tuning knob to cryogenic near-field experiments on emerging phenomena in 2D materials and moiré heterostructures.



